Preliminary study of the criticality monitoring method based on the simulation for the activity ratio of short half-life noble-gas fission products from fuel debris

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi; Kanno, Ikuo

Journal of Nuclear Science and Technology, 8 Pages, 2024/00

https://doi.org/10.1080/00223131.2023.2300773

Void reactivity in lead and bismuth sample reactivity experiments at Kyoto University Critical Assembly

Pyeon, C. H.*; Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro

Nuclear Science and Engineering, 197(11), p.2902 - 2919, 2023/11

https://doi.org/10.1080/00295639.2023.2172311

Sample reactivity and void reactivity experiments are carried out in the solid-moderated and solid-reflected cores at the Kyoto University Critical Assembly (KUCA) with the combined use of aluminum (Al), lead (Pb) and bismuth (Bi) samples, and Al spacers simulating the void. MCNP6.2 eigenvalue calculations together with JENDL-4.0 provide good accuracy of sample reactivity with the comparison of experimental results; also experimental void reactivity is attained by using MCNP6.2 together with JENDL-4.0 and ENDF/B-VII.1 with a marked accuracy of relative difference between experiments and calculations. Uncertainty quantification of sample reactivity and void reactivity is acquired by using the sensitivity coefficients based on MCNP6.2/ksen and covariance library data of SCALE6.2 together with ENDF/B-VII.1, arising from the impact of uncertainty induced by Al, Pb and Bi cross sections. A series of reactivity analyses with the Al spacer simulating the void demonstrates the means of analyzing the void in the solid-moderated and solid-reflected cores at KUCA

Elemental analysis and radioactivity evaluation of aerosols generated during heating of simulated fuel debris; The Urasol project in the framework of Fukushima Daiichi fuel debris removal

Tsubota, Yoichi; Porcheron, E.*; Journeau, C.*; Delacroix, J.*; Suteau, C.*; Lallot, Y.*; Bouland, A.*; Roulet, D.*; Mitsugi, Takeshi

Proceedings of International Conference on Environmental Remediation and Radioactive Waste Management (ICEM2023) (Internet), 6 Pages, 2023/10

https://doi.org/10.1115/ICEM2023-110064

In order to safely remove fuel debris from the Fukushima Daiichi Nuclear Power Station (1F), it is necessary to quantitatively evaluate radioactive airborne particulate generated by the cutting of nuclear fuel debris. We fabricated Uranium-bearing simulated fuel debris (SFD) with In/Ex-Vessel compositions and evaluated the physical and chemical properties of aerosols generated by heating the SFDs. Based on these results, we estimated the isotopic composition and radioactivity of aerosols produced when 1F-Unit2 fuel debris is laser cut, which is a typical example of a heating method. Plutonium, mainly Pu,Am, and Cm were found to be the alpha nuclide, and Pu, Cs-Ba, and Sr-Y were found to be the beta nuclide of interest.

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-2, JRR-3 and Hot laboratory

Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; Konda, Miki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2023-002, 81 Pages, 2023/05

JAEA-Data-Code-2023-002.pdf:3.0MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2, JRR-3 and Hot laboratory facilities. In this report, we summarized the radioactivity concentrations of 20 radionuclides (H, C, Cl, Co, Ni, Sr, Nb, Tc, Ag, I, Cs, Eu, Eu, U, U, Pu, Pu, Pu, Am, Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2020.

JAEA/ISCN delayed gamma-ray spectroscopy inverse Monte Carlo development status

Rodriguez, D.; Rossi, F.

Proceedings of INMM & ESARDA Joint Annual Meeting 2023 (Internet), 9 Pages, 2023/05

Validation of feedback reactivity evaluation models for plant dynamics analysis code during unprotected loss of heat sink event in sodium-cooled fast reactors

Yoshimura, Kazuo; Doda, Norihiro; Igawa, Kenichi*; Tanaka, Masaaki; Yamano, Hidemasa

Journal of Nuclear Engineering and Radiation Science, 9(2), p.021601_1 - 021601_9, 2023/04

https://doi.org/10.1115/1.4055328

Feedback reactivity automatically caused by radial expansion of the core is known as one of the inherent safety features in a sodium-cooled fast reactor (SFR). In order to validate the evaluation models of the reactivity feedback equipped in the in-house plant dynamics analysis code named Super-COPD, the benchmark analyses for the unprotected loss of heat sink (ULOHS) tests of BOP-302R and BOP-301 in an experimental SFR, EBR-II were conducted and the applicability of the evaluation method for the reactivity feedback was indicated during the ULOHS even, by comparing the numerical results and the experimental data.

Study on safety characteristics of a sodium-cooled fast reactor with negative void reactivity during initiating phase in severe accident

Ishida, Shinya; Fukano, Yoshitaka; Tobita, Yoshiharu; Okano, Yasushi

Proceedings of 2023 International Congress on Advanced in Nuclear Power Plants (ICAPP 2023) (Internet), 8 Pages, 2023/04

TRU oxide sample reactivity worths measured in the FCA-IX assemblies with systematically changed neutron energy spectra

Fukushima, Masahiro; Okajima, Shigeaki*; Mukaiyama, Takehiko*

Journal of Nuclear Science and Technology, 20 Pages, 2023/00

https://doi.org/10.1080/00223131.2023.2240872

A series of integral experiments was conducted to evaluate the fission and the capture cross- sections of transuranic (TRU) nuclides at the fast critical facility FCA of the Japan Atomic Energy Agency (JAEA). The experiments were carried out using seven uranium-fueled assemblies of the FCA. The neutron energy spectra of the core regions were adjusted so as to change from an intermediate neutron spectrum to a fast neutron spectrum on an assembly-by-assembly basis. The integral data measured with these experimental configurations provide some neutron energy characteristics: 1) fission rate ratios (FRRs) of Np, Pu, Pu, Am, Am, and Cm relative to Pu by using absolutely calibrated fission chambers, 2) small sample reactivity worths (SRWs) of Np, Pu, Pu, Am, and Am where oxide powders of around 15 to 20 grams were used, 3) criticalities, and 4) spectral indices such as fission rate ratios of U relative to U. In this paper, details of the SRW measurements are reported, and the latest Japanese Evaluated Nuclear Data Library JENDL-5 is tested by using the integral data obtained in systematically varied neutron energy spectra.

Impact of uncertainty reduction on lead-bismuth coolant in accelerator-driven system using sample reactivity experiments

Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro; Pyeon, C. H.*; Yamamoto, Akio*; Endo, Tomohiro*

Nuclear Science and Engineering, 20 Pages, 2023/00

https://doi.org/10.1080/00295639.2023.2246779

In this study, we have demonstrated that data assimilation using lead and bismuth sample reactivities measured in the Kyoto University Critical Assembly A-core can successfully reduce the uncertainty of the coolant void reactivity in accelerator-driven systems derived from inelastic-scattering cross-sections of lead and bismuth. We re-evaluated and highlighted the experimental uncertainties and correlations of the sample reactivities for the data assimilation formula. We used the MCNP6.2 code to evaluate the sample reactivities and their uncertainties, and performed data assimilation using the reactor analysis code system MARBLE. The high-sensitivity coefficients of the sample reactivities to lead and bismuth allowed us to reduce the cross-section-induced uncertainty of the void reactivity of the accelerator-driven system from 6.3% to 4.8%, achieving a provisional target accuracy of 5% in this study. Furthermore, we demonstrated that the uncertainties arising from other dominant factors, such as minor actinides and steel, can be effectively reduced by using integral experimental data sets for the unified cross-section dataset ADJ2017.

Reactivity estimation based on the linear equation of characteristic time profile of power in subcritical quasi-steady state

Yamane, Yuichi

Journal of Nuclear Science and Technology, 59(11), p.1331 - 1344, 2022/11

https://doi.org/10.1080/00223131.2022.2053221

The reactivity was estimated from a time profile of neutron count rate or a simulated data in a quasi-steady state after sudden change of reactivity or external neutron source strength. The estimation was based on the equation of power in subcritical quasi-steady state. The purpose of the study is to develop the method of timely reactivity estimation from complicated time profile of neutron count rate. The developed method was applied to the data simulating neutron count rate created by using one-point kinetics code, AGNES, and Poisson-distributed random noise and to the transient subcritical experiment data measured by using TRACY. The result shows that the difference of the estimated and reference value was within about 5% or less for ( -1) for simulated data and within about 7% or less for -1.4 and -3.1 for the experimental data. It was also shown that the possibility of the reactivity estimation several ten seconds after the status change.